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Electronic ground-state hysteresis under magnetic field in GdMn2O5

2023/07/12 by V, Balédent, A., Vaunat, S., Petit +4
#FOS: Physical sciences #Materials Science (cond-mat.mtrl-sci) #Strongly Correlated Electrons (cond-mat.str-el)

paper · doi:10.48550/arxiv.2307.06247

Abstract

In this paper, we investigate the physical properties of the type II multiferroic GdMn2O5 material by means of neutrons scattering, electric polarization and magnetization measurements. A complex (T,H) phase diagram shows up, with especially a field induced magnetic transition around 12 T at low temperature. The high field phase is accompanied by an additional electric polarization along both the a and b directions, as authorized by symmetry, but never observed experimentally up to now. While the magnetic properties recover their initial states after driving the field back to zero, the polarization along a shows a significant increase. This behavior is observed for all directions of the magnetic field. It constitutes a novel and striking manifestation of the magneto-electric coupling, resulting in the establishment of a new ground state at zero magnetic field.

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