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Witnessing Quantum Entanglement Using Resonant Inelastic X-ray Scattering

2024/04/08 by Tianhao Ren, Ren, Tianhao, Yao Shen +20 · 7 citations
Physics and Astronomy · #Crystallography and Radiation Phenomena #FOS: Physical sciences #Quantum Physics (quant-ph) #Strongly Correlated Electrons (cond-mat.str-el)

paper · pdf · doi:10.48550/arxiv.2404.05850

openalex publication_date 2024/04/08 · openalex created_date 2024/04/11 · openalex updated_date 2026/08/01

Abstract

Although entanglement is both a central ingredient in our understanding of quantum many-body systems and an essential resource for quantum technologies, we only have a limited ability to quantify entanglement in real quantum materials. Thus far, entanglement metrology in quantum materials has been limited to measurements involving Hermitian operators, such as the detection of spin entanglement using inelastic neutron scattering. Here, we devise a method to extract the quantum Fisher information (QFI) from non-Hermitian operators and formulate an entanglement witness for resonant inelastic x-ray scattering (RIXS). Our approach is then applied to the model iridate dimer system Ba3CeIr2O9 and used to directly test for entanglement of the electronic orbitals between neighboring Ir sites. We find the entanglement can be detected if we account for the expected symmetries, parity, and electron number conservation, of the dimer system. We also consider the roles that the incident and outgoing x-ray polarizations and the incident photon energy play in entanglement detection. Our protocol provides a new handle for entanglement detection in quantum materials.

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