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Experimental Approach to the Thermodynamics of the Pure Two-Dimensional Spin-1/2 Triangular Lattice Antiferromagnet in Ba8CoNb6O24

2016/12/15 by Yi Cui, Cui, Y., J. Dai +23
Materials Science · Physics and Astronomy · #Advanced Condensed Matter Physics #FOS: Physical sciences #Magnetic and transport properties of perovskites and related materials #Physics of Superconductivity and Magnetism #Strongly Correlated Electrons (cond-mat.str-el) #Superconductivity (cond-mat.supr-con)

paper · pdf · doi:10.48550/arxiv.1612.05217

openalex publication_date 2016/12/15 · openalex created_date 2025/10/10 · openalex updated_date 2026/07/28

Abstract

Frustrated quantum magnets pose well-defined questions concerning quantum fluctuation effects and the nature of the many-body wavefunction, which challenge theory, numerics, experiment and materials synthesis. The S = 1/2 triangular-lattice antiferromagnet (TLAF) presents a case where classical order is strongly suppressed by quantum fluctuations, leading to extensive renormalization of physical properties at all energy scales. However, purely two-dimensional (2D) models are difficult to realise in the 3D world and their physics is controlled by the Mermin-Wagner theorem, which describes the dominant effects of additional thermal fluctuations. Here we report the magnetic properties Ba8CoNb6O24, whose Co2+ions have an effective spin 1/2 and construct a regular TLAF with very large interlayer spacing. We find no magnetic ordering down to 0.028 K, strong low-energy spin fluctuations in qualitative agreement with theoretical analysis and a diverging correlation length, all indicating a Mermin-Wagner trend towards zero-temperature ordering in this ideal 2D system.

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