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The exchange coupling between the valence electrons of the fullerene cage and the electrons of the N atoms in N@C60-1,3

2009/09/22 by L. Udvardi, Udvardi, L.
Chemistry · Engineering · Physics and Astronomy · #Atomic and Molecular Physics #FOS: Physical sciences #Fullerene Chemistry and Applications #Mesoscale and Nanoscale Physics (cond-mat.mes-hall) #Molecular Junctions and Nanostructures #Other Condensed Matter (cond-mat.other) #cond-mat.mes-hall #cond-mat.other

paper · pdf · doi:10.48550/arxiv.0909.3939

arxiv created 2009/09/22 · openalex publication_date 2009/09/22 · arxiv updated 2009/12/01 · openalex created_date 2025/10/10 · openalex updated_date 2026/07/28

Abstract

MCSCF calculations are performed in order to determine the exchange coupling between the 2p electrons of the N atom and the LUMOs of the fullerene cage in the case of mono- and tri-anions of N@C60. The exchange coupling resulted by our calculations is large compared to the hyperfine interaction. The strong coupling can explain the missing EPR signal of the nitrogen in paramagnetic anions.

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