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Colossal Magnetocapacitance Effect and Multiferroism of Polycrystalline La0.2Pb0.7Fe12O19

2016/03/15 by Tan, Guo-Long, Haohao Sheng, Sheng, Hao-Hao
Engineering · Materials Science · #FOS: Physical sciences #Magnetic and transport properties of perovskites and related materials #Magneto-Optical Properties and Applications #Materials Science (cond-mat.mtrl-sci) #Multiferroics and related materials

paper · pdf · doi:10.48550/arxiv.1603.04508

openalex publication_date 2016/03/15 · openalex created_date 2016/06/24 · openalex updated_date 2026/07/28

Abstract

The mutual control of the electric and magnetic properties of a multiferroic solid is of fundamental and great technological importance. We report here on the colossal magnetoelectric coupling effect of polycrystalline La0.2Pb0.7Fe12O19. A large classic ferroelectric hysteresis loop with full saturation and a strong magnetic hysteresis loop were observed simultaneously in polycrystalline La0.2Pb0.7Fe12O19 due to the coexistence of an off-centered FeO6 octahedron in its unit cell and electron spins in the partially filled 3d orbits of the Fe3+ ions. The coupling voltage and capacity demonstrate giant oscillations, along with magnetic field; the maximum magnetocapacitance ratio exceeds 1.9E5 at 80 Hz. The substitution of La ions with Pb ions progressively stabilized the conical spin structure, which gave rise to the spin-current induced capacity oscillations upon magnetic field.

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