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Photon Counting Statistics for Single Molecule Spectroscopy

2001/04/11 by Eli Barkai, Barkai, Eli, YounJoon Jung +4
Biochemistry, Genetics and Molecular Biology · Physics and Astronomy · #Advanced Fluorescence Microscopy Techniques #Quantum optics and atomic interactions #Spectroscopy and Quantum Chemical Studies #cond-mat.mes-hall #cond-mat.stat-mech

paper · pdf · doi:10.48550/arxiv.cond-mat/0104188

arxiv created 2001/04/11 · arxiv updated 2009/11/30

Abstract

We present a general relation between Mandel's Q parameter describing variance of number of photons emitted from a single molecule and a three time correlation function describing a spectral diffusion process the molecule is undergoing. For a prototype of such a stochastic process an exact solution is found which exhibits rich types of physical behaviors.

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