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Effect of uniaxial stress on helimagnetic phases in the square-lattice itinerant magnet EuAl4

2025/11/10 by Gen, Masaki, Nomoto, Takuya, Saito, Hiraku +5
Materials Science · Physics and Astronomy · #Advanced Thermoelectric Materials and Devices #FOS: Physical sciences #Magnetic and transport properties of perovskites and related materials #Materials Science (cond-mat.mtrl-sci) #Rare-earth and actinide compounds #Strongly Correlated Electrons (cond-mat.str-el)

paper · doi:10.48550/arxiv.2511.07079

openalex publication_date 2025/11/10 · openalex created_date 2025/11/12 · openalex updated_date 2026/07/28

Abstract

We investigate uniaxial-stress effects on the magnetic phase diagram of the square-lattice itinerant magnet EuAl4, where strong coupling among spin, lattice, and charge produces a variety of helimagnetic phases, including rhombic and square skyrmion lattices. Combining resistivity and magnetization measurements with neutron scattering, we find that compressive stresses of only several tens of megapascal along [010] enhance antiferromagnetic character and shorten the magnetic modulation period in the lowest-temperature single-Q spiral state, thereby driving the critical temperatures and fields of multiple phases to higher values. First-principles calculations show that increasing orthorhombic lattice distortion deforms the Fermi surface relevant to the magnetism, providing compelling evidence that Fermi-surface nesting plays a crucial role in stabilizing the helical magnetic modulations in EuAl4.

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