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Robust Coherent Control of Bimolecular Collisions beyond the Ultracold Regime

2023/06/23 by Adrien Devolder, Devolder, Adrien, Paul Brumer +3
Computer Science · Physics and Astronomy · #Atomic Physics (physics.atom-ph) #Atomic and Subatomic Physics Research #Chemical Physics (physics.chem-ph) #Cold Atom Physics and Bose-Einstein Condensates #FOS: Physical sciences #Quantum Information and Cryptography #Quantum Physics (quant-ph)

paper · pdf · doi:10.48550/arxiv.2306.13470

openalex publication_date 2023/06/23 · openalex created_date 2023/06/28 · openalex updated_date 2026/07/28

Abstract

Quantum coherent control of bimolecular collisions beyond the ultracold regime can face a major challenge due to the incoherent addition of different partial wave contributions to the total scattering cross section. These contributions become increasingly numerous as the collision energy increases, leading to a loss of overall control. Here, we overcome this limitation by leveraging the recently discovered Partial Wave Phase Locking (PWPL) effect, which synchronizes the oscillations of all partial wave contributions. By using rigorous quantum scattering calculations, we demonstrate that PWPL enables coherent control of spin exchange in ion-atom collisions, far outside the ultracold regime, even with as many as 5000 partial wave contributions. The predicted extent of control is sufficient to be measurable in cold atom-ion hybrid experiments.

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