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High Compression Blue-Detuned Magneto-Optical Trap of Polyatomic Molecules

2024/04/04 by Christian Hallas, Grace K. Li, Hallas, Christian +9 · 2 citations
Engineering · Physics and Astronomy · #Atomic Physics (physics.atom-ph) #FOS: Physical sciences #Molecular Junctions and Nanostructures #Photonic and Optical Devices #Quantum optics and atomic interactions

paper · pdf · doi:10.48550/arxiv.2404.03636

openalex publication_date 2024/04/04 · openalex created_date 2024/04/06 · openalex updated_date 2026/07/28

Abstract

We demonstrate a blue-detuned magneto-optical trap (MOT) of a polyatomic molecule, calcium monohydroxide (CaOH). We identify a novel MOT frequency configuration that produces high spatial compression of the molecular cloud. This high compression MOT achieves a cloud radius of 59(5)~μm and a peak density of 8(2) × 108~cm-3, the highest reported density for a molecular MOT to date. We compare our experimental studies of blue-detuned MOTs for CaOH and compare with Monte-Carlo simulations, finding good agreement.

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