2018/02/22 by M. Zhu, P. G. Li, Zhu, M. +15
Materials Science · Physics and Astronomy · #Advanced Condensed Matter Physics #FOS: Physical sciences #Magnetic and transport properties of perovskites and related materials #Multiferroics and related materials #Strongly Correlated Electrons (cond-mat.str-el)
paper · pdf · doi:10.48550/arxiv.1802.08293
openalex publication_date 2018/02/22 · openalex created_date 2025/10/10 · openalex updated_date 2026/07/28
Sr4Ru3O10, the n = 3 member of the Ruddlesden-Popper type ruthenate Srn+1RunO3n+1, is known to exhibit a peculiar metamagnetic transition in an in-plane magnetic field. However, the nature of both the temperature- and field-dependent phase transitions remains as a topic of debate. Here, we have investigated the magnetic transitions of Sr4Ru3O10 via single-crystal neutron diffraction measurements. At zero field, we find that the system undergoes a ferromagnetic transition with both in-plane and out-of-plane magnetic components at Tc ~ 100 K. Below T* ~ 50 K, the magnetic moments incline continuously toward the out-of-plane direction. At T ~ 1.5 K, where the spins are nearly aligned along the c axis, a spin reorientation occurs above a critical field Bc, giving rise to a spin component perpendicular to the plane defined by the field direction and the c axis. We suggest that both the temperature- and field-driven spin reorientations are associated with a change in the magnetocrystalline anisotropy, which is strongly coupled to the lattice degrees of freedom. This study elucidates the long-standing puzzles on the zero-field magnetic orders of Sr4Ru3O10 and provides new insights into the nature of the field-induced metamagnetic transition.