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Molecular impurities interacting with a many-particle environment: from helium droplets to ultracold gases

2017/03/20 by Mikhail Lemeshko, Richard Schmidt, Lemeshko, Mikhail +1
Physics and Astronomy · #Atomic Physics (physics.atom-ph) #Atomic and Molecular Clusters (physics.atm-clus) #Atomic and Subatomic Physics Research #Chemical Physics (physics.chem-ph) #Cold Atom Physics and Bose-Einstein Condensates #FOS: Physical sciences #Mesoscale and Nanoscale Physics (cond-mat.mes-hall) #Quantum Gases (cond-mat.quant-gas) #Quantum, superfluid, helium dynamics

paper · pdf · doi:10.48550/arxiv.1703.06753

openalex publication_date 2017/03/20 · openalex created_date 2025/10/10 · openalex updated_date 2026/07/28

Abstract

In several settings of physics and chemistry one has to deal with molecules interacting with some kind of an external environment, be it a gas, a solution, or a crystal surface. Understanding molecular processes in the presence of such a many-particle bath is inherently challenging, and usually requires large-scale numerical computations. Here, we present an alternative approach to the problem - that based on the notion of the angulon quasiparticle. We show that molecules rotating inside superfluid helium nanodroplets and Bose-Einstein Condensates form angulons, and therefore can be described by straightforward solutions of a simple microscopic Hamiltonian. Casting the problem in the language of angulons allows not only to tremendously simplify it, but also to gain insights into the origins of the observed phenomena and to make predictions for future experimental studies.

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