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Robust analytic continuation approach to many-body GW calculations

2019/12/13 by Ivan Duchemin, Xavier Blase, Duchemin, Ivan +1 · 3 citations
Physics and Astronomy · #Advanced Chemical Physics Studies #FOS: Physical sciences #Materials Science (cond-mat.mtrl-sci) #Quantum, superfluid, helium dynamics #Spectroscopy and Quantum Chemical Studies

paper · pdf · doi:10.48550/arxiv.1912.06459

openalex publication_date 2019/12/13 · openalex created_date 2025/10/10 · openalex updated_date 2026/07/28

Abstract

The analytic continuation of the GW self-energy from the imaginary to the real energy axis is a central difficulty for approaches exploiting the favourable properties of response functions at imaginary frequencies. Within a scheme merging contour-deformation and analytic-continuation techniques, we show on the basis of extensive calculations for large molecular sets that it is preferable to perform an analytic continuation of the dynamically screened Coulomb potential W rather than the much more structured self-energy operator. The case of states lying far away from the gap, including core states, is addressed by generalizing the analytic continuation scheme, accounting further for quasiparticle lifetimes.

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