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Enhancement of Chirality-Induced Spin Selectivity by Strong Electron Correlations

2024/05/07 by Xu, Meng, Chen, Yan · 2 citations
#Biological Physics (physics.bio-ph) #FOS: Physical sciences #Mesoscale and Nanoscale Physics (cond-mat.mes-hall) #Strongly Correlated Electrons (cond-mat.str-el)

paper · doi:10.48550/arxiv.2405.04316

Abstract

Chirality-induced spin selectivity is a spin-splitting phenomenon from a helical structure with a considerably effective spin-orbit coupling. This unexpectedly large spin-splitting phenomenon has been experimentally observed in chiral organic molecules, which typically show a weak spin-orbit coupling. To understand this, we use the renormalized mean-field theory and Landauer-Büttiker formulas to study the transport properties of single-stranded DNA in the presence of strong electron correlation. It shows a significant spin polarization of 46.5% near the Coulomb repulsion limit, which explains the extremely high spin polarization observed in experiments. Compared to systems without electron correlation, the averaged spin polarization in this case is 2 to 4 times greater across various system sizes. Furthermore, the parameter dependence of the spin polarization and the underlying Metal-Insulator transition are studied.

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