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Giant Raman Intensity Modulation in Pristine Carbon Nanotubes

2009/05/05 by Adam W. Bushmaker, Adam Bushmaker, Vikram V. Deshpande +9
Biochemistry, Genetics and Molecular Biology · Materials Science · Physics and Astronomy · #Carbon Nanotubes in Composites #FOS: Physical sciences #Graphene research and applications #Mesoscale and Nanoscale Physics (cond-mat.mes-hall) #Spectroscopy Techniques in Biomedical and Chemical Research #Strongly Correlated Electrons (cond-mat.str-el) #cond-mat.mes-hall #cond-mat.str-el

paper · pdf · doi:10.48550/arxiv.0905.0694

arxiv created 2009/05/05 · openalex publication_date 2009/05/05 · arxiv updated 2009/12/01 · openalex created_date 2025/10/10 · openalex updated_date 2026/07/28

Abstract

Large variations of up to two orders of magnitude are observed in the Raman intensity of pristine, suspended quasi-metallic single-walled carbon nanotubes in response to applied gate potentials. No change in the resonance condition is observed, and all Raman bands exhibit the same changes in intensity, regardless of phonon energy or laser excitation energy. The effect is not observed in semiconducting nanotubes. The electronic energy gaps correlate with the drop in the Raman intensity, and the recently observed Mott insulating behavior is suggested as a possible explanation for this effect.

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