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Novel approach to nonlinear susceptibility

2003/11/17 by M. Combescot, Combescot, M., O. Betbeder-Matibet +5
Computer Science · Engineering · Physics and Astronomy · #FOS: Physical sciences #Mechanical and Optical Resonators #Mesoscale and Nanoscale Physics (cond-mat.mes-hall) #Photonic and Optical Devices #Quantum Information and Cryptography #Strongly Correlated Electrons (cond-mat.str-el) #cond-mat.mes-hall #cond-mat.str-el

paper · pdf · doi:10.48550/arxiv.cond-mat/0311387

arxiv created 2003/11/17 · openalex publication_date 2003/11/17 · arxiv updated 2009/12/01 · openalex created_date 2025/10/10 · openalex updated_date 2026/07/28

Abstract

The calculation of the third order susceptibility still is a long standing fundamental problem of particular importance in nonlinear nanooptics: Indeed, cancellation of size-dependent terms coming from uncorrelated excitations is expected, but up to now shown for very simple Hamiltonians only. Using a many-body theory recently developed to handle interacting close-to-bosons, we prove it here for arbitrary H. This new formalism actually provides the first clean way to calculate nonlinear susceptibilities, with results different from previous ones.

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