2016/06/07 by Sergio Gómez‐Graña, Aurélie Le Beulze, Gomez-Graña, Sergio +33
Engineering · Materials Science · Physics and Astronomy · #FOS: Physical sciences #Materials Science (cond-mat.mtrl-sci) #Mesoscale and Nanoscale Physics (cond-mat.mes-hall) #Metamaterials and Metasurfaces Applications #Photonic Crystals and Applications #Plasmonic and Surface Plasmon Research
paper · doi:10.48550/arxiv.1606.02105
openalex publication_date 2016/06/07 · openalex created_date 2025/10/10 · openalex updated_date 2026/07/28
Hierarchical self-assembly arranges nanostructures at different length scales. It gradually becomes an effective method of fabricating artificial metamaterials from composite nanostructures tailored for a particular response. Hierarchical self-assembly overcomes shortcomings of "top-down" methods by significantly reducing fabrication time and making it possible to form bulk materials. Here we report an application of hierarchical self-assembly of metal nanoparticles for the creation of the first isotropic optical metamaterial with strong artificial magnetism in blue light. We have used colloidal self-assembly to create artificial "nanomolecules" that generate the desired magnetic response and microfluidic self-assembly to produce a bulk metastructure. We demonstrate that the magnetic response of the final material is accurately described by an isotropic magnetic permeability that satisfies the principle of locality. Our approach unlocks the fabrication of large volumes of composite nanomaterials. Moreover, the spatial disorder inherent to this "bottom-up" method holds the key to solving the non-locality problem. The technique can be readily extended to the future generations of low-loss optical metamaterials made of dielectric nano-blocks to bypass the limitations of optical losses associated with plasmonic resonances in noble metals.