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Dimension-free Ergodicity of Path Integral Molecular Dynamics

2023/07/13 by Ye, Xuda, Zhou, Zhennan
#37A30 #81S40 #82B31 #Computational Physics (physics.comp-ph) #FOS: Mathematics #FOS: Physical sciences #Numerical Analysis (math.NA) #Probability (math.PR) #Quantum Physics (quant-ph)

paper · doi:10.48550/arxiv.2307.06510

Abstract

The quantum thermal average plays a central role in describing the thermodynamic properties of a quantum system. Path integral molecular dynamics (PIMD) is a prevailing approach for computing quantum thermal averages by approximating the quantum partition function as a classical isomorphism on an augmented space, enabling efficient classical sampling, but the theoretical knowledge of the ergodicity of the sampling is lacking. Parallel to the standard PIMD with N ring polymer beads, we also study the Matsubara mode PIMD, where the ring polymer is replaced by a continuous loop composed of N Matsubara modes. Utilizing the generalized Γ calculus, we prove that both the Matsubara mode PIMD and the standard PIMD have uniform-in-N ergodicity, i.e., the convergence rate towards the invariant distribution does not depend on the number of modes or beads N.

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