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Electrical Control of Optically Active Single Spin Qubits in ZnSe

2025/12/25 by Amirehsan Alizadehherfati, Yuxi Jiang, Alizadehherfati, Amirehsan +15 · 1 citation
Computer Science · Physics and Astronomy · #FOS: Physical sciences #Quantum Information and Cryptography #Quantum Physics (quant-ph) #Quantum and electron transport phenomena #Quantum optics and atomic interactions

paper · doi:10.48550/arxiv.2512.21462

openalex publication_date 2025/12/25 · openalex created_date 2025/12/30 · openalex updated_date 2026/07/28

Abstract

Electrons bound to shallow donors in ZnSe quantum wells are promising candidates for optically addressable spin qubits and single-photon sources. However, their optical coherence and indistinguishability are often limited by spectral broadening arising from charge fluctuations in the local environment. Here, we report electrical control of single donor qubits in ZnSe quantum wells. The applied field induces a DC Stark shift that tunes the emission energy over a range exceeding 30 times the inhomogeneous linewidth, effectively compensating for emitter-to-emitter variations. Concurrently, the field stabilizes trap occupancy, yielding a twofold reduction in optical linewidth and the suppression of spectral wandering. A statistical model based on trap dynamics qualitatively reproduces these observations and elucidates the mechanism of field-assisted charge noise suppression. Our results identify electrical control as a versatile pathway to significantly improve optical and spin addressability.

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