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Surface Rashba-Edelstein Spin-Orbit Torque Revealed by Molecular Self-Assembly

2020/04/21 by Satoshi Haku, Haku, Satoshi, Atsushi Ishikawa +9
Engineering · Physics and Astronomy · #FOS: Physical sciences #Magnetic properties of thin films #Materials Science (cond-mat.mtrl-sci) #Mesoscale and Nanoscale Physics (cond-mat.mes-hall) #Molecular Junctions and Nanostructures #Quantum and electron transport phenomena

paper · pdf · doi:10.48550/arxiv.2004.09852

openalex publication_date 2020/04/21 · openalex created_date 2025/10/10 · openalex updated_date 2026/07/28

Abstract

We report the observation of a spin-orbit torque (SOT) originating from the surface Rashba-Edelstein effect. We found that the SOT in a prototypical spin-orbitronic system, a Pt/Co bilayer, can be manipulated by molecular self-assembly on the Pt surface. This evidences that the Rashba spin-orbit coupling at the Pt surface generates a sizable SOT, which has been hidden by the strong bulk and interface spin-orbit coupling. We show that the molecular tuning of the surface Rashba-Edelstein SOT is consistent with density functional theory calculations. These results illustrate the crucial role of the surface spin-orbit coupling in the SOT generation, which alters the landscape of metallic spin-orbitronic devices.

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