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Strain-Gradient-Driven Decoupling of Thermal Suppression from Anisotropy in \beta-Ga2O3

2025/09/30 by Zhang, Guangwu, Xiang, Xing, Qian, Ziyan +7 · 1 citation
#Atomic Physics (physics.atom-ph) #FOS: Physical sciences #Materials Science (cond-mat.mtrl-sci)

paper · doi:10.48550/arxiv.2509.26412

Abstract

Strain gradients, ubiquitous in flexible devices and epitaxial nanostructures, are a major blind spot for thermal transport in \beta-Ga2O3. We establish that strain gradient unlocks a thermal conductivity (k) suppression mechanism fundamentally more potent than uniform strain: moderate uniaxial gradients (0.6%/nm) suppress k by 32-37% (27-30%) in thin films (nanowires), intensifying to 43.3% with biaxial gradients. This reduction far exceeds that from equivalent uniform strain and surpasses benchmark materials like silicon and BAs. Critically, a surprising decoupling emerges: while 3% uniform strain alters thermal anisotropy by ~25%, strain gradient strongly suppresses k with preserving this ratio. Mechanistically, strain gradients-induced symmetry breaking and enhanced mode coupling anisotropically activate forbidden scattering channels, making gradient-driven scattering dominant over intrinsic phonon scattering below 6.25 THz. These findings redefine non-uniform strain from a parasitic flaw into a powerful design tool for engineering thermal isolation and heat flux in next-generation flexible and high-power \beta-Ga2O3 electronics.

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