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Bioinspired Synergistic Texture and Color Modulation Enabled by Surface Instability of Cholesteric Liquid Crystal Elastomers

2025/08/05 by Yang, Xiao, Sim, Jay, Huang, Wenbin +1
#Applied Physics (physics.app-ph) #FOS: Physical sciences

paper · doi:10.48550/arxiv.2508.03870

Abstract

Certain cephalopods can dynamically camouflage by altering both skin texture and color to match their surroundings. Inspired by this capability, we present a cholesteric liquid crystal elastomer-liquid crystal elastomer (CLCE-LCE) bilayer capable of simultaneous, reversible modulation of surface texture and structural color through programmable wrinkling. By tuning the bilayer's fabrication parameters, on-demand wrinkle morphologies and color combinations are achieved. Spatially selective UV curing allows localized surface textures, while chemical patterning of the CLCE layer enables region-specific color responses, expanding the design space for multifunctional, spatially encoded optical materials. The CLCE-LCE bilayer enables dynamic thermal regulation by tuning light absorption through synergistically modulating surface morphology and color. Notably, this system achieves strain-dependent multiscale encoding via multistep selective UV curing, revealing distinct visual content under different applied strains. This work establishes a versatile platform that merges surface instabilities with tunable structural coloration, advancing intelligent materials with programmable, strain-responsive surface and optical properties.

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