2013/05/20 by Z. -T. Lu, Zheng‐Tian Lu, Lu, Z. -T. +29 · 1 citation
Earth and Planetary Sciences · Environmental Science · Physics and Astronomy · #FOS: Physical sciences #Geophysics (physics.geo-ph) #Groundwater and Isotope Geochemistry #Isotope Analysis in Ecology #Marine Biology and Ecology Research #physics.geo-ph
paper · pdf · doi:10.48550/arxiv.1305.4608
openalex publication_date 2013/05/20 · arxiv created 2013/08/23 · arxiv updated 2013/08/26 · openalex created_date 2025/10/10 · openalex updated_date 2026/07/28
The noble gas radionuclides, including 81Kr (half-life = 229,000 yr), 85Kr (11 yr), and 39Ar (269 yr), possess nearly ideal chemical and physical properties for studies of earth and environmental processes. Recent advances in Atom Trap Trace Analysis (ATTA), a laser-based atom counting method, have enabled routine measurements of the radiokrypton isotopes, as well as the demonstration of the ability to measure 39Ar in environmental samples. Here we provide an overview of the ATTA technique, and a survey of recent progress made in several laboratories worldwide. We review the application of noble gas radionuclides in the geosciences and discuss how ATTA can help advance these fields, specifically determination of groundwater residence times using 81Kr, 85Kr, and 39Ar; dating old glacial ice using 81Kr; and an 39Ar survey of the main water masses of the oceans, to study circulation pathways and estimate mean residence times. Other scientific questions involving deeper circulation of fluids in the Earth's crust and mantle also are within the scope of future applications. We conclude that the geoscience community would greatly benefit from an ATTA facility dedicated to this field, with instrumentation for routine measurements, as well as for research on further development of ATTA methods.