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Rheology and microrheology of deformable droplet suspensions

2018/08/30 by M. Foglino, A. N. Morozov, Foglino, M. +4
Chemical Engineering · Materials Science · Physics and Astronomy · #FOS: Physical sciences #Material Dynamics and Properties #Pickering emulsions and particle stabilization #Rheology and Fluid Dynamics Studies #Soft Condensed Matter (cond-mat.soft) #cond-mat.soft

paper · pdf · doi:10.48550/arxiv.1808.10361

arxiv created 2018/08/30 · openalex publication_date 2018/08/30 · arxiv updated 2018/08/31 · openalex created_date 2025/10/10 · openalex updated_date 2026/07/28

Abstract

Dense suspensions of soft colloidal particles display a broad range of physical and rheological properties which are still far from being fully understood. To elucidate the role of deformability on colloidal flow, we employ computer simulations to measure the apparent viscosity of a system of droplets of variable surface tension subjected to a pressure-driven flow. We confirm that our suspension generically undergoes discontinuous shear thinning, and determine the dependence of the onset of the discontinuity on surface tension. We find that the effective viscosity of the suspension is mainly determined by a capillary number. We present active microrheology simulations, where a single droplet is dragged through the suspension. These also show a dynamical phase transition, analogous to the one associated with discontinuous shear thinning in our interpretation. Such a transition is signalled by a discontinuity in the droplet velocity versus applied force.

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