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High resolution Hall measurements across the VO2 metal-insulator transition reveal impact of spatial phase separation

2015/10/19 by Tony Yamin, Yamin, Tony, Yakov M. Strelniker +3
Engineering · Materials Science · Physics and Astronomy · #Advanced Memory and Neural Computing #Ga2O3 and related materials #Transition Metal Oxide Nanomaterials #cond-mat.mtrl-sci #cond-mat.str-el

paper · pdf · doi:10.48550/arxiv.1510.05414

15 p, 4 figures

arxiv created 2015/10/19 · arxiv updated 2015/10/20

Abstract

Many strongly correlated transition metal oxides exhibit a metal-insulator transition (MIT), the manipulation of which is essential for their application as active device elements. However, such manipulation is hindered by lack of microscopic understanding of mechanisms involved in these transitions. A prototypical example is VO2, where previous studies indicated that the MIT resistance change correlate with changes in carrier density and mobility. We studied the MIT using Hall measurements with unprecedented resolution and accuracy, simultaneously with resistance measurements. Contrast to prior reports, we find that the MIT is not correlated with a change in mobility, but rather, is a macroscopic manifestation of the spatial phase separation which accompanies the MIT. Our results demonstrate that, surprisingly, properties of the nano-scale spatially-separated metallic and semiconducting domains actually retain their bulk properties. This study highlights the importance of taking into account local fluctuations and correlations when interpreting transport measurements in highly correlated systems.

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