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Time-domain interferences as the source of electron-ion entanglement in Rabi-dressed photoemission

2025/07/08 by Léonardo Rico, Morgan Berkane, Rico, Léonardo +9
Biochemistry, Genetics and Molecular Biology · Physics and Astronomy · #Advanced Electron Microscopy Techniques and Applications #Atomic Physics (physics.atom-ph) #Atomic and Molecular Physics #FOS: Physical sciences #Laser-Matter Interactions and Applications #Quantum Physics (quant-ph)

paper · pdf · doi:10.48550/arxiv.2507.05850

openalex publication_date 2025/07/08 · openalex created_date 2025/10/10 · openalex updated_date 2026/07/28

Abstract

We investigate bipartite entanglement between a photoelectron and its parent ion when the latter undergoes Rabi oscillations, following the recent experiment of [Nandi et al. Science Advances 10, eado0668 (2024)]. Using numerical simulations on a model atom, we show that this entanglement results from ionization events occurring at different times, with the photoelectron leaving the ion in distinct superpositions of internal states due to the Rabi coupling. Our interpretation brings forward the possibility to access the purity of the photoion state from photoelectron spectra. Furthermore, we demonstrate a tomographic reconstruction of the dressed ionic state dynamics from the observable spectra.

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