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Understanding the degradation of a model Si-anode in Li-ion battery at the atomic-scale

2022/07/17 by Kim, Se-Ho, Dong, Kang, Zhao, Huan +7 · 3 citations
#FOS: Physical sciences #Materials Science (cond-mat.mtrl-sci)

paper · doi:10.48550/arxiv.2207.08154

Abstract

Si-anodes have long been candidates thanks to an expected ten-fold increase in capacity compared to graphite. However, details of the mechanisms governing their degradation remain elusive, hindering science-guided development of long-lived Si-based anodes. Here we demonstrate how the latest developments in cryo-atom probe tomography enable the in-depth analysis of the electrode and electrolyte, and their interface at atomic-level.

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