Anisotropy-driven quantum capacitance in multi-layered black phosphorus

2017/08/08 by Parijat Sengupta, Sengupta, Parijat, Shaloo Rakheja +1
Materials Science · Physics and Astronomy · #2D Materials and Applications #Topological Materials and Phenomena #Photorefractive and Nonlinear Optics

paper · pdf · doi:10.48550/arxiv.1708.02350

Abstract

We report analytic results on quantum capacitance (C_q) measurements and their optical tuning in dual-gated device with potassium-doped multi-layered black phosphorous (BP) as the channel material. The two-dimensional (2D) layered BP is highly anisotropic with a semi-Dirac dispersion marked by linear and quadratic contributions. The C_q calculations mirror this asymmetric arrangement. A further increase to the asymmetry and consequently C_q is predicted by photon-dressing the BP dispersion. To achieve this and tune C_q in a field-effect transistor (FET), we suggest a configuration wherein a pair of electrostatic (top) and optical (back) gates clamp a BP channel. The back gate shines an optical pulse to rearrange the dispersion of the 2D BP. Analytic calculations are done with Floquet Hamiltonians in the off-resonant regime. The value of such C_q calculations, in addition, to its role in adjusting the current drive of an FET is discussed in context of metal-insulator and topological phase transitions and enhancements to the thermoelectric figure of merit.

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