2025/10/28 by Zhenhao Gong, Zhen-Hao Gong, Zhi-Hao Wei +8
Physics and Astronomy · Materials Science · Engineering · #Nonlinear Photonic Systems #Nonlocal and gradient elasticity in micro/nano structures #Nonlinear Optical Materials Studies
paper · pdf · doi:10.1103/515g-qjq8
In nonlinear transport, the quantum-geometric effects can generate higher-harmonic voltages in response to a driving current, which has defined a fast-moving field of intense interest. However, in realistic materials where disorder scattering also contributes to nonlinear transport, identifying the geometric mechanisms remains a challenge. In particular, a theoretical framework for data analysis is still lacking for nonlinear transport at any order. Here, we develop a mechanism-resolved and symmetry-guided framework for identifying mechanisms of third-order nonlinear transport in disordered materials. We find a total of 20 mechanisms of third-order nonlinear transport, by treating quantum-geometric and disorder-mediated mechanisms on an equal footing. More importantly, we propose a protocol of data analysis that combines symmetry diagnosis of magnetic point groups and scaling law of relation between the third-order nonlinear Hall conductivity and linear longitudinal conductivity. We identify characteristic fingerprints in the scaling-law weights, which allow the mechanisms to be quantitatively distinguished in experiments. We have applied the protocol to identify the geometric mechanisms in materials with and without time-reversal symmetry, including 2D materials, topological materials, and altermagnets. The theory can be generalized to arbitrary orders of nonlinear transport, further promoting nonlinear transport as a probe of geometric effects and phase transitions in quantum materials.