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Revealing spin-flip two-level systems using ultra-thin film superconducting resonators

2024/12/20 by Zi‐Qing Huang, Huang, Zi-Qing, Shu-Kun Ye +19
Physics and Astronomy · #FOS: Physical sciences #Magnetic properties of thin films #Mesoscale and Nanoscale Physics (cond-mat.mes-hall) #Physics of Superconductivity and Magnetism #Quantum Physics (quant-ph) #Quantum and electron transport phenomena

paper · pdf · doi:10.48550/arxiv.2412.15856

openalex publication_date 2024/12/20 · openalex created_date 2024/12/24 · openalex updated_date 2026/07/28

Abstract

Material disorders are one of the major sources of noise and loss in solid-state quantum devices, whose behaviors are often modeled as two-level systems (TLSs) formed by charge tunneling between neighboring sites. However, the role of their spins in tunneling and its impact on device performance remain highly unexplored. In this work, employing ultra-thin TiN superconducting resonators, we reveal anomalous TLS behaviors by demonstrating an unexpected increase in resonant frequency at low magnetic fields. Furthermore, a spin-flip TLS model is proposed, in which an effective spin-orbit coupling is generated by inhomogeneous local magnetic fields from defect spins. This mechanism mixes charge tunnelings and spin flips, quantitatively reproducing the observed frequency-field relationship and its temperature dependence. This work deepens the understanding of spin-dependent TLS behaviors, offering the possibility of magnetically engineering noise and loss in solid-state quantum devices.

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